论文标题

连贯的GE(1-X)SN(X)/GE异质结构中载体寿命的磁光测定

Magneto-optical determination of the carrier lifetime in coherent Ge(1-x)Sn(x)/Ge heterostructures

论文作者

Vitiello, Elisa, Rossi, Simone, Broderick, Christopher A., Gravina, Giorgio, Balocchi, Andrea, Marie, Xavier, O'Reilly, Eoin P., Myronov, Maksym, Pezzoli, Fabio

论文摘要

我们提出了一项对压缩性GE(1-X)SN(X)膜中载体动力学的磁光研究,其SN组成在SI(001)虚拟底物上的毯子GE上具有最高10%的外延生长。我们利用稳态激发下的Hanle效应来研究存在外部磁场的旋转依赖性光学转变。这使我们能够直接访问光学诱导的载体种群的动态。我们的方法指出,在低温温度下,相干GE(1-X)SN(X)中光生载体的有效寿命发生在子-NS时间尺度上。在辐射寿命的模型估计值的支持下,我们的测量表明载体重组由非​​辐射过程主导。因此,我们的结果提供了中心信息,以促进这种新型直接差距IV材料系统中对载体动力学的基本理解。这些知识可以是寻求GE(1-X)SN(X)基于功能设备的垫脚石。

We present a magneto-optical study of the carrier dynamics in compressively strained Ge(1-x)Sn(x) films having Sn compositions up to 10% epitaxially grown on blanket Ge on Si (001) virtual substrates. We leverage the Hanle effect under steady-state excitation to study the spin-dependent optical transitions in presence of an external magnetic field. This allowed us to obtain direct access to the dynamics of the optically-induced carrier population. Our approach singled out that at cryogenic temperatures the effective lifetime of the photogenerated carriers in coherent Ge(1-x)Sn(x) occurs in the sub-ns time scale. Supported by a model estimate of the radiative lifetime, our measurements indicate that carrier recombination is dominated by non-radiative processes. Our results thus provide central information to advance the fundamental understanding of carrier kinetics in this novel direct-gap group-IV material system. Such knowledge can be a stepping stone in the quest for the implementation of Ge(1-x)Sn(x)-based functional devices.

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