论文标题
双层元面,用于增强的光子上转换
Double-Layer Metasurface for Enhanced Photon Up-Conversion
论文作者
论文摘要
我们提出了通过堆叠硅纳米盘阵列和硅光子晶体平板而获得的双层介电元表,彼此之间具有相等的周期性。我们专注于对元图的谐振激发产生的电近场增强效应的研究,并在数值和实验上研究其光学特性。我们发现,与传统的单层结构相比,多层跨额的主要差异似乎是在雷利木异常中:它们被分为多种不同的模式,这些模式本身在光谱上宽广。作为概念的证明,我们涵盖了一个具有灯笼掺杂的上转换层层的双层跨表面,并研究了其与1550 nm光激发的相互作用。我们通过使用堆叠的元表面而不是平面底物观察到2.7倍增强的上转化光致发光,尽管只有大约1%的上转材料暴露于增强的近场。确定了两种机制来解释这种行为:首先,当跨表情刺激跨场时增强了近场,第二,当元表面重定向将光重定向到高角度衍射顺序时,在粒子层中的全部反射捕获。这些结果为低阈值,尤其是将来的太阳能和生物传感应用中的宽带光子上转换铺平了道路。
We present a double-layer dielectric metasurface obtained by stacking a silicon nanodisc array and a silicon photonic crystal slab with equal periodicity on top of each other. We focus on the investigation of electric near-field enhancement effects occurring at resonant excitation of the metasurface and study its optical properties numerically and experimentally. We find that the major difference in multi-layer metasurfaces when compared to conventional single-layer structures appears to be in Rayleigh-Wood anomalies: they are split into multiple different modes which are themselves spectrally broadened. As a proof of concept we cover a double-layer metasurface with a lanthanide-doped up-conversion particle layer and study its interaction with a 1550 nm photoexcitation. We observe a 2.7-fold enhancemed up-conversion photoluminescence by using the stacked metasurface instead of a planar substrate, although only around 1% of the up-conversion material is exposed to enhanced near-fields. Two mechanisms are identified explaining this behavior: First, enhanced near-fields when exciting the metasurface resonantly, and second, light trapping by total internal reflection in the particle layer when the metasurface redirects light into high-angle diffraction orders. These results pave the way for low-threshold and, in particular, broadband photon up-conversion in future solar energy and biosensing applications.