论文标题
辐射诱导的基于苯基聚合物闪烁体的变化中的剂量速率效应
Dose rate effects in radiation-induced changes to phenyl-based polymeric scintillators
论文作者
论文摘要
介绍了由Eljen Technology Company生产的塑料闪烁杆产生的电离辐射对各种基质材料,掺杂剂浓度,荧光(EJ-200和EJ-260),抗氧化剂浓度,闪烁剂厚度,剂量和剂量率的影响。使用Alpha源和光电层管测量照射前后的光输出,以及分光光度计的光传输。假设以剂量的指数下降,则使用指数剂量常数$ d $量化光输出的变化。 $ d $值的初级和二次掺杂浓度为1和2倍,而默认制造商的浓度为0、1和2倍的抗氧化剂浓度。 $ d $值大致取决于所有材料的剂量率在2.2 gy/hr和70 Gy/hr之间的剂量率的对数。 For EJ-200 polyvinyltoluene-based (PVT) scintillator, the dose constant is approximately linear in the logarithm of the dose rate up to 3400 Gy/hr, while for polystyrene-based (PS) scintillator or for both materials with EJ-260 fluors, it remains constant or decreases (depending on doping concentration) above about 100 Gy/hr.厚度不同的杆和不同荧光的杆的结果表明,对初始光输出的损害比闪烁体厚度$ \ leq1 $ cm的颜色中心形成效果更大。对于蓝色闪光灯(EJ-200),传输测量值表示荧光的损害。我们还发现,虽然PVT比PS的剂量速率更高,而EJ-200荧光的剂量速率高于约100 Gy/hr,但在较低剂量速率和EJ-260荧光的情况下,它们显示出相似的损害。
Results on the effects of ionizing radiation on the signal produced by plastic scintillating rods manufactured by Eljen Technology company are presented for various matrix materials, dopant concentrations, fluors (EJ-200 and EJ-260), anti-oxidant concentrations, scintillator thickness, doses, and dose rates. The light output before and after irradiation is measured using an alpha source and a photomultiplier tube, and the light transmission by a spectrophotometer. Assuming an exponential decrease in the light output with dose, the change in light output is quantified using the exponential dose constant $D$. The $D$ values are similar for primary and secondary doping concentrations of 1 and 2 times, and for antioxidant concentrations of 0, 1, and 2 times, the default manufacturer's concentration. The $D$ value depends approximately linearly on the logarithm of the dose rate for dose rates between 2.2 Gy/hr and 70 Gy/hr for all materials. For EJ-200 polyvinyltoluene-based (PVT) scintillator, the dose constant is approximately linear in the logarithm of the dose rate up to 3400 Gy/hr, while for polystyrene-based (PS) scintillator or for both materials with EJ-260 fluors, it remains constant or decreases (depending on doping concentration) above about 100 Gy/hr. The results from rods of varying thickness and from the different fluors suggest damage to the initial light output is a larger effect than color center formation for scintillator thickness $\leq1$ cm. For the blue scintillator (EJ-200), the transmission measurements indicate damage to the fluors. We also find that while PVT is more resistant to radiation damage than PS at dose rates higher than about 100 Gy/hr for EJ-200 fluors, they show similar damage at lower dose rates and for EJ-260 fluors.