论文标题

结构性130-K相过渡和ht-ce $ _2 $ rh $ rh $ _2 $ ga的两个离子近代状态的出现,$^{69,71} $ ga ga ga nou nou nou nou nou nou nou nou nou nou nou nou nou nucu Quadrupole共振

Structural 130-K Phase Transition and Emergence of a Two-Ion Kondo State in HT-Ce$_2$Rh$_2$Ga Explored by $^{69,71}$Ga Nuclear Quadrupole Resonance

论文作者

Yamamoto, Sh., Fujii, T., Luther, S., Yasuoka, H., Sakai, H., Bärtl, F., Ranjith, K. M., Rosner, H., Wosnitza, J., Strydom, A. M., Kühne, H., Baenitz, M.

论文摘要

我们已经研究了微观磁性特性,130-K相变的性质以及最近合成的化合物CE $ _2 $ RH $ _2 $ GA中的基态,并使用$^{69,71} $ ga ga ga nou nuco nuco nuco nuco nucu nou nucu nucu nuco nucu nuco nucu nucode Quadrupole rupole rupole resonance(nqr)。 NQR光谱清楚地显示出在$ t_t $ $ \ sim $ 130 K处的异常相转换,从而将高温单个NQR线分解为两条清晰解析的NQR线,提供了两个结晶性不相同的GA位点的证据。 NQR频率与频带结构的全面计算非常吻合。 Our NQR results indicate the absence of magnetic or charge order down to 0.3 K. The temperature dependence of the spin-lattice relaxation rate, 1/$T_1$, shows three distinct regimes, with onset temperatures at $T_t$ and 2 K. The temperature-independent 1/$T_1$, observed between $T_t$ and 2 K, crosses over to a Korringa process, 1/$T_1$ $\propto$ $ t $,低于$ \ sim $ 2 K,这证明了一种罕见的两离子围栏场景:该系统在两个不同的GA站点中进入2.0的密集近相干状态,而0.8 K。

We have studied the microscopic magnetic properties, the nature of the 130-K phase transition, and the ground state in the recently synthesized compound Ce$_2$Rh$_2$Ga by use of $^{69,71}$Ga nuclear quadrupole resonance (NQR). The NQR spectra clearly show an unusual phase transition at $T_t$ $\sim$ 130 K yielding a splitting of the high-temperature single NQR line into two clearly resolved NQR lines, providing evidence for two crystallographically inequivalent Ga sites. The NQR frequencies are in good agreement with fully-relativistic calculations of the band structure. Our NQR results indicate the absence of magnetic or charge order down to 0.3 K. The temperature dependence of the spin-lattice relaxation rate, 1/$T_1$, shows three distinct regimes, with onset temperatures at $T_t$ and 2 K. The temperature-independent 1/$T_1$, observed between $T_t$ and 2 K, crosses over to a Korringa process, 1/$T_1$ $\propto$ $T$, below $\sim$ 2 K, which evidences a rare two-ion Kondo scenario: the system goes into a dense Kondo coherent state at 2.0 and 0.8 K for the two different Ga sites.

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